Advances in Chemical Physics, Vol. 83 by I. Prigogine, Stuart A. Rice

By I. Prigogine, Stuart A. Rice

Each one quantity during this sequence is dedicated to aiding the reader to acquire common information regarding various themes in chemical physics. This quantity comprises dialogue of high-temperature superconductors, time-resolved optical checks of digital geometric part improvement and masses extra.

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4). Therefore, regardless of molecular orientation, there is nonzero vibrational displacement only along the q,-mode at t = 0. By writing Eq. 3) explicitly as q,,) = - r,,IMw,( 1 - sin’@ cos’@), we is less see that the range of orientations within which the magnitude of than a certain value, say d m , decreases with increasing pulse energy. In practice, the nonresonant pulse pair will be replaced with a sequence of such pairs, spaced at the ground state pseudorotational period, in order to drive the pseudorotation to large amplitude and discriminate against other low frequency modes [30,49-521.

L. J. Boya, and B. Kendrick, Phys. Rev. A 43, 1206 (1991). 7. N. F. Scherer, A. J. Ruggiero, M. Du, and G. R. Fleming, J . Chem. Phys. 93, 856 ( 1990). 8. (a) N. F. Scherer, R. J . Carlson, A. Matro, M. Du, A. J. Ruggiero, V. Romero-Rochin, J. A. Cina, G. R. Fleming, and S. A. Rice, J . Chem. Phys. 95, 1487 (1991); (b) N. F. Scherer, A. Matro, R. J. Carlson, M. Du. L. D. Ziegler, J. A. Cina, and G. R. Fleming, J . Chem. Phys. 196, 4180 (1992). 9. ( a ) H . Metiu and V. Engel, J . O p t . SOC. Am.

4) apply to both resonant and nonresonant processes. For passive processes, first of all, the phase matching condition may not always be satisfied. For the phase mismatched case, Ak; # 0, it is evident from Eq. 4) that W:)(r; w,) oscillates along r with the period equal to the coherence length, I < .

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